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Construction of MoS2/Tubular-like g-C3N4 Composite Photocatalyst for Improved Visible-Light Photocatalytic Hydrogen Production from Seawater
Author NameAffiliationE-mail
SHI Wei-Long School of Material Science and Engineering, Beihua University, Jilin, Jilin 132013, China
School of Material Science and Engineering, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212003, China 
 
YANG Shuang School of Material Science and Engineering, Beihua University, Jilin, Jilin 132013, China  
WANG Jing-Bo School of Material Science and Engineering, Beihua University, Jilin, Jilin 132013, China  
LIN Xue School of Material Science and Engineering, Beihua University, Jilin, Jilin 132013, China jlsdlinxue@126.com 
GUO Feng School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212013, China gfeng0105@126.com 
SHI Jun-You School of Material Science and Engineering, Beihua University, Jilin, Jilin 132013, China bhsjy64@163.com 
Abstract: In this work, the development of efficient and stable photocatalyst has been the central topic of scientific research. Herein, MoS2 nanosheets/tubular-like g-C3N4 (MS/TCN) composite photocatalysts with two dimension/one dimension (2D/1D) nanostructure were fabricated through a facile solvothermal method for photocatalytic hydrogen production from seawater under visible light irradiation, exhibiting enhanced photocatalytic performance in comparison of single MS or TCN. Among of them, MS/TCN-0.5 sample (0.5%(w/w) MoS2) showed optimum H2 evolution rate of 85.1 μmol·h-1 and possessed outstanding stability (no significant decrease after 4 cycles). The enhanced photocatalytic activity of MS/TCN composite photocatalyst can be attributed to the fact that the loading of 2D MS, as a cocatalyst, promotes the transfer of photo-induced electron and improves the separation efficiency of electron-hole pairs of 1D TCN.
Keywords: photocatalysis  hydrogen production  carbon nitride  molybdenum disulfide
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SHI Wei-Long,YANG Shuang,WANG Jing-Bo,LIN Xue,GUO Feng,SHI Jun-You.Construction of MoS2/Tubular-like g-C3N4 Composite Photocatalyst for Improved Visible-Light Photocatalytic Hydrogen Production from Seawater[J].Chinese Journal of Inorganic Chemistry,2020,36(8):1582-1592.
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Chinese Journal of Inorganic Chemistry